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Rat liver homogenates catalyze a two-electron reduction of hypoxanthine to xanthine which can be blocked by adding purine nucleoside phosphorylase. The formation of xanthine from hypoxanthine is inhibited by allopurinol and xanthine oxidase, thus identifying this reaction as the first step in purine salvage. Prior treatment of the tissue with hypoxanthine guanine phosphoribosyltransferase (EC 2.4.2.8) was found to enhance the nucleoside reducing activity. The purification of this enzyme preparation is described. The flavoenzyme purified to homogeneity (molecular weight of 46,000) has an absolute requirement for iron, a reduced requirement for both flavin and FAD, and a very narrow pH optimum of 8.6. The enzyme is not immunologically cross-reactive with xanthine oxidase. The nucleoside reductase may serve a regulatory function in that the level of this enzyme in different organs should influence the utilization of adenine nucleotides in the pentose phosphate pathway, the de novo synthesis of purine nucleotides, and the activity of purine nucleoside phosphorylase.Q:

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